yes
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smartly smartly, as in The young soldier saluted smartly.
No, it's an adjective.An adverb form would be smartly.
Smarter.First find the base of smartly: smart. Now imagine the word for 'more smart.' Smarter. If you wanted to continue that pattern, and find the superlative, you would imagine the word for 'most smart,' smartest.(If you want to make a comparative adverb, you simply say more adverb; for example, more smartly.)
Mrs Tan likes to dress smartly whenever she goes out.
Smartly?